Bogoliubov transformations and exact isolated solutions for simple non-adiabatic Hamiltonians

We present a new method for finding isolated exact solutions of a class of non-adiabatic Hamiltonians of relevance to quantum optics and allied areas. Central to our approach is the use of Bogoliubov transformations of the bosonic fields in the models. We demonstrate the simplicity and efficiency of this method by applying it to the Rabi Hamiltonian.Comment: LaTeX, 16 pages, 1 figure. Minor additions and journal re

Exact isolated solutions for the two-photon Rabi Hamiltonian

The two-photon Rabi Hamiltonian is a simple model describing the interaction of light with matter, with the interaction being mediated by the exchange of two photons. Although this model is exactly soluble in the rotating-wave approximation, we work with the full Hamiltonian, maintaining the non-integrability of the model. We demonstrate that, despite this non-integrability, there exist isolated, exact solutions for this model analogous to the so-called Juddian solutions found for the single-photon Rabi Hamiltonian. In so doing we use a Bogoliubov transformation of the field mode, as described by the present authors in an earlier publication.Comment: 15 Pages, 1 Figure, Latex, minor change

Phase Transitions in the Spin-Half J_1--J_2 Model

The coupled cluster method (CCM) is a well-known method of quantum many-body theory, and here we present an application of the CCM to the spin-half J_1--J_2 quantum spin model with nearest- and next-nearest-neighbour interactions on the linear chain and the square lattice. We present new results for ground-state expectation values of such quantities as the energy and the sublattice magnetisation. The presence of critical points in the solution of the CCM equations, which are associated with phase transitions in the real system, is investigated. Completely distinct from the investigation of the critical points, we also make a link between the expansion coefficients of the ground-state wave function in terms of an Ising basis and the CCM ket-state correlation coefficients. We are thus able to present evidence of the breakdown, at a given value of J_2/J_1, of the Marshall-Peierls sign rule which is known to be satisfied at the pure Heisenberg point (J_2 = 0) on any bipartite lattice. For the square lattice, our best estimates of the points at which the sign rule breaks down and at which the phase transition from the antiferromagnetic phase to the frustrated phase occurs are, respectively, given (to two decimal places) by J_2/J_1 = 0.26 and J_2/J_1 = 0.61.Comment: 28 pages, Latex, 2 postscript figure

Systematic Inclusion of High-Order Multi-Spin Correlations for the Spin-121\over2 XXZXXZ Models

We apply the microscopic coupled-cluster method (CCM) to the spin-$1\over2$ $XXZ$ models on both the one-dimensional chain and the two-dimensional square lattice. Based on a systematic approximation scheme of the CCM developed by us previously, we carry out high-order {\it ab initio} calculations using computer-algebraic techniques. The ground-state properties of the models are obtained with high accuracy as functions of the anisotropy parameter. Furthermore, our CCM analysis enables us to study their quantum critical behavior in a systematic and unbiased manner.Comment: (to appear in PRL). 4 pages, ReVTeX, two figures available upon request. UMIST Preprint MA-000-000

High-Order Coupled Cluster Method Calculations for the Ground- and Excited-State Properties of the Spin-Half XXZ Model

In this article, we present new results of high-order coupled cluster method (CCM) calculations, based on a N\'eel model state with spins aligned in the $z$-direction, for both the ground- and excited-state properties of the spin-half {\it XXZ} model on the linear chain, the square lattice, and the simple cubic lattice. In particular, the high-order CCM formalism is extended to treat the excited states of lattice quantum spin systems for the first time. Completely new results for the excitation energy gap of the spin-half {\it XXZ} model for these lattices are thus determined. These high-order calculations are based on a localised approximation scheme called the LSUB$m$ scheme in which we retain all $k$-body correlations defined on all possible locales of $m$ adjacent lattice sites ($k \le m$). The ``raw'' CCM LSUB$m$ results are seen to provide very good results for the ground-state energy, sublattice magnetisation, and the value of the lowest-lying excitation energy for each of these systems. However, in order to obtain even better results, two types of extrapolation scheme of the LSUB$m$ results to the limit $m \to \infty$ (i.e., the exact solution in the thermodynamic limit) are presented. The extrapolated results provide extremely accurate results for the ground- and excited-state properties of these systems across a wide range of values of the anisotropy parameter.Comment: 31 Pages, 5 Figure

A new method for the determination of thin film porosity

Internal reflection spectroscopy may be used to determine presence of water in thin film pores. Presence of water in such pores is function of relative humidity and pore size. Thus, one can determine pore size by controlling humidity. Fluids with surface tension different from that of water can be used to detect pores

Influence of quantum fluctuations on zero-temperature phase transitions between collinear and noncollinear states in frustrated spin systems

We study a square-lattice spin-half Heisenberg model where frustration is introduced by competing nearest-neighbor bonds of different signs. We discuss the influence of quantum fluctuations on the nature of the zero-temperature phase transitions from phases with collinear magnetic order at small frustration to phases with noncollinear spiral order at large frustration. We use the coupled cluster method (CCM) for high orders of approximation (up to LSUB6) and the exact diagonalization of finite systems (up to 32 sites) to calculate ground-state properties. The role of quantum fluctuations is examined by comparing the ferromagnetic-spiral and the antiferromagnetic-spiral transition within the same model. We find clear evidence that quantum fluctuations prefer collinear order and that they may favour a first order transition instead of a second order transition in case of no quantum fluctuations.Comment: 6 pages, 6 Postscipt figures; Accepted for publication in Phys. Rev.

Highly frustrated spin-lattice models of magnetism and their quantum phase transitions: A microscopic treatment via the coupled cluster method

We outline how the coupled cluster method of microscopic quantum many-body theory can be utilized in practice to give highly accurate results for the ground-state properties of a wide variety of highly frustrated and strongly correlated spin-lattice models of interest in quantum magnetism, including their quantum phase transitions. The method itself is described, and it is shown how it may be implemented in practice to high orders in a systematically improvable hierarchy of (so-called LSUB$m$) approximations, by the use of computer-algebraic techniques. The method works from the outset in the thermodynamic limit of an infinite lattice at all levels of approximation, and it is shown both how the "raw" LSUB$m$ results are themselves generally excellent in the sense that they converge rapidly, and how they may accurately be extrapolated to the exact limit, $m \rightarrow \infty$, of the truncation index $m$, which denotes the {\it only} approximation made. All of this is illustrated via a specific application to a two-dimensional, frustrated, spin-half $J^{XXZ}_{1}$--$J^{XXZ}_{2}$ model on a honeycomb lattice with nearest-neighbor and next-nearest-neighbor interactions with exchange couplings $J_{1}>0$ and $J_{2} \equiv \kappa J_{1} > 0$, respectively, where both interactions are of the same anisotropic $XXZ$ type. We show how the method can be used to determine the entire zero-temperature ground-state phase diagram of the model in the range $0 \leq \kappa \leq 1$ of the frustration parameter and $0 \leq \Delta \leq 1$ of the spin-space anisotropy parameter. In particular, we identify a candidate quantum spin-liquid region in the phase space

Spin-1/2 J1J_{1}-J2J_{2} Heisenberg model on a cross-striped square lattice

Using the coupled cluster method (CCM) we study the full (zero-temperature) ground-state (GS) phase diagram of a spin-half ($s=1/2$) $J_{1}$-$J_{2}$ Heisenberg model on a cross-striped square lattice. Each site of the square lattice has 4 nearest-neighbour exchange bonds of strength $J_{1}$ and 2 next-nearest-neighbour (diagonal) bonds of strength $J_{2}$. The $J_{2}$ bonds are arranged so that the basic square plaquettes in alternating columns have either both or no $J_{2}$ bonds included. The classical ($s \rightarrow \infty$) version of the model has 4 collinear phases when $J_{1}$ and $J_{2}$ can take either sign. Three phases are antiferromagnetic (AFM), showing so-called N\'{e}el, double N\'{e}el and double columnar striped order respectively, while the fourth is ferromagnetic. For the quantum $s=1/2$ model we use the 3 classical AFM phases as CCM reference states, on top of which the multispin-flip configurations arising from quantum fluctuations are incorporated in a systematic truncation hierarchy. Calculations of the corresponding GS energy, magnetic order parameter and the susceptibilities of the states to various forms of valence-bond crystalline (VBC) order are thus carried out numerically to high orders of approximation and then extrapolated to the (exact) physical limit. We find that the $s=1/2$ model has 5 phases, which correspond to the four classical phases plus a new quantum phase with plaquette VBC order. The positions of the 5 quantum critical points are determined with high accuracy. While all 4 phase transitions in the classical model are first order, we find strong evidence that 3 of the 5 quantum phase transitions in the $s=1/2$ model are of continuous deconfined type